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Krause was selected in the second round of the NFL draft by the Redskins (1964-1967) in 1964. He led the NFL in interceptions with 12 as a rookie and was named 1st Team All Pro. He played the majority of his career for the Vikings (1968-1979). In his first season as a Viking, he intercepted passes in 6 consecutive games. His 10 interceptions in 1975 remains a club record and he still holds the NFL record for career interceptions with 81.